Design of simulated-gas calibration source and self-attenuation correction methods for radioactive noble gas measurement with HPGe detector.

In this study, to achieve accurate measurement of radioactive noble gas and enhance the precision of efficiency calibration, a relatively low-cost and low-density simulated-gas calibration source (SGCS) was produced from polyurethane foam with a density of ρ = 0.098 g cm-3. Using SGCS with a Marinelli beaker geometry, the efficiency calibration was applied to a BE5030, 50.5% relative efficiency HPGe detector in an energy range of 59.54 keV∼1836.06 keV. Then, taking the 81 keV gamma-ray emitted by 133Xe as an example, due to the density difference between the SGCS and the 133Xe gas sample, it is necessary to correct for self-attenuation effects. Therefore, a semi-empirical function for self-attenuation correction was established by using LabSOCS software and XCOM. Upon validation, the relative deviation of efficiency calibration values between the SGCS and the LabSOCS of 133Xe under the density of 0.001 g cm-3 to 0.01 g cm-3 was about 3%. After using the self-attenuation correction method established in this study, the results verified a good consistency of the efficiency calculated by SGCS and LabSOCS software.

The calibration of transfer standards for the measurement of 222Rn at NIM.

A high-purity germanium (HPGe) gamma-ray spectrometer and an Alpha-GUARD radon monitor are the activity and activity concentration transfer standards of 222Rn, respectively. The gaseous 222Rn standard source traceable to the NIM's absolute standardization apparatus of 222Rn was developed for calibrating these transfer standards. The calibration results of HPGe detector at three different distances show that the uncertainties of experimental efficiency are less than 0.77% (k = 1). Meanwhile, the Monte Carlo (MC) simulation was carried out at wider distances range for the HPGe calibration as well, and the deviation at same three distances between experiments and simulations results is within ±3.0%. The advantage of calibration using MC simulation and the possible reasons for the deviation were discussed in detail in this article. In addition, a reference activity concentration environment based on the gaseous 222Rn standard source was also developed to calibrate the radon monitor, and the typical uncertainty for calibration factor of Alpha-GUARD radon monitor could be reduced to 1.9% (k = 1).